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ЖУРНАЛЫ // Оптика и спектроскопия // Архив

Оптика и спектроскопия, 2020, том 128, выпуск 8, страница 1193 (Mi os346)

Нанофотоника

Charge transfer from lead sulfide quantum dots to MoS$_{2}$ nanoplatelets

I. D. Skurlov, A. S. Mudrak, A. V. Sokolova, S. A. Cherevkov, M. A. Baranov, A. Dubavik, P. S. Parfenov, A. P. Litvin

ITMO University, St. Petersburg, Russia

Аннотация: The research interest in the transition metal dichalcogenides (TMD) has been reborn a few years ago. This had happened due to the remarkable properties of monolayered TMD (e. g. high carrier mobility and high exciton binding energy) and due to the development of the exfoliation methods. Photoconductive MoS$_{2}$-based devices spectral range can be expanded to the NIR by coupling them with PbS QDs. However, this requires extensive knowledge about the the charge and energy transfer processes in such systems. In this paper, we investigate charge transfer between PbS QDs and MoS$_{2}$ nanoplatelets (NPls). Using the PL decay analysis, we show how the charge transfer efficiency changes with the distance between the QDs and NPls, as well as with QD size. Last, we demonstrate that the addition of the MoS$_{2}$ NPLs increases the photoconductive response for up to an order of magnitude, as compared to the bare QD.

Ключевые слова: transition metal dichalcogenides, quantum dots, charge transfer, lead sulfide, molybdenum disulfide.

Поступила в редакцию: 18.01.2020
Исправленный вариант: 18.01.2020
Принята в печать: 20.04.2020

Язык публикации: английский


 Англоязычная версия: Optics and Spectroscopy, 2020, 128:8, 1236–1240

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