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Fizika Tverdogo Tela, 2024 Volume 66, Issue 1, Pages 94–102 (Mi ftt10218)

Magnetism, spintronics

Yttrium influence on magnetic properties and hyperfine interactions in multicomponent substitution alloys (Dy$_{1-x}$Y$_x$)$_{0.8}$Sm$_{0.2}$Fe$_2$

Z. S. Umkhaevaa, V. S. Rusakovb, T. V. Gubaidulinab, A. Yu. Karpenkovc, I. S. Tereshinab, N. Yu. Pankratovb, I. M. Alieva

a Complex Research Institute named after Kh. I. Ibragimov, Russian Academy of Sciences, Grozny, Russia
b Lomonosov Moscow State University, Moscow, Russia
c Tver State University, Tver, Russia

Abstract: The paper presents the results of investigation of structure, magnetic properties and superfine interactions in multicomponent alloys based on rare-earth elements $(R)$, Sm and their analogue Y of $R$Fe$_2$ stoichiometry. To obtain new multicomponent alloys, a complex type of substitution in the rare-earth sublattice was used, namely, weakly magnetic samarium atoms at a fixed concentration of 20 at.% were first introduced into the dysprosium sublattice, followed by non-magnetic yttrium atoms at the values of the substitution parameter $x$ = 0, 0.2, 0.4, 0.6, 0.8, 1.0. This type of substitution, first of all, leads to the competition of exchange interactions between magnetically active ions in a wide temperature region of their magnetic ordering. The competition also leads to a number of unique magnetic phase transformations in the resulting alloys, including the phenomenon of magnetic compensation of the rare-earth and 3d sublattice, as well as spin reorientation. The values of the main parameters of Mossbauer spectra on $^{57}$Fe nuclei in (Dy$_{1-x}$Y$_x$)$_{0.8}$Sm$_{0.2}$Fe$_2$alloys and their dependence on yttrium concentration at $T$ = 300 K have been determined. The field dependences of magnetostriction in fields up to 12 kOe have been investigated.

Keywords: Laves phases, magnetization, Curie temperature, magnetic moment, Mossbauer effect, hyperfine interactions.

Received: 06.10.2023
Revised: 23.10.2023
Accepted: 13.11.2023

DOI: 10.61011/FTT.2024.01.56943.220



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