Abstract:
DC-induced generation of the reflected second harmonic is experimentally observed on the surface of a centrosymmetric silicon single crystal. A direct current with a surface density of jmax ~ 103 A/cm2 violates the symmetry of the electron distribution function and induces the optical second harmonic with an intensity corresponding to the dipole quadratic susceptibility χ(2)d(jmax) ~ 3 × 10−15 m/V.