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JOURNALS // Pis'ma v Zhurnal Èksperimental'noi i Teoreticheskoi Fiziki // Archive

Pis'ma v Zh. Èksper. Teoret. Fiz., 2025 Volume 121, Issue 1, Pages 72–77 (Mi jetpl7414)

METHODS OF PHYSICAL INVESTIGATION

Highly correlated electronic state in the ferrimagnetic quadruple perovskite CuCu$_3$Fe$_2$Re$_2$O$_{12}$

A. I. Poteryaevab, Z. V. Pchelkinaba, S. V. Streltsovab, Y. Longc, V. Yu. Irkhina

a Institute of Metal Physics, Russian Academy of Sciences, Yekaterinburg, 620108 Russia
b Department of Theoretical Physics and Applied Mathematics, Ural Federal University, Yekaterinburg, 620002 Russia
c Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing, 100190 China

Abstract: Recently synthesized quadruple perovskite CuCu$_3$Fe$_2$Re$_2$O$_{12}$ possesses strong ferromagnetism and unusual electron properties, including enhanced electronic specific heat. Application of the first principles electronic structure approaches unambiguously shows importance of the many-body effects in this compound. While CuCu$_3$Fe$_2$Re$_2$O$_{12}$ is half-metallic ferrimagnet in the DFT+U method, in the density functional theory (DFT) combined with the dynamical mean-field theory (DMFT) it appears to be a metal. Strong electronic correlations leads to a renormalization of electronic spectrum and formation of incoherent states close to the Fermi level. Electronic specific heat and magnetic properties obtained in the DFT+DMFT approach are in better agreement with available experimental data than derived by other band structure techniques.

Received: 05.11.2024
Revised: 18.11.2024
Accepted: 18.11.2024

DOI: 10.31857/S0370274X25010116


 English version:
Journal of Experimental and Theoretical Physics Letters, 2025, 121:1, 67–71


© Steklov Math. Inst. of RAS, 2025