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Optics and Spectroscopy, 2024 Volume 132, Issue 7, Pages 740–746 (Mi os1225)

Spectroscopy of condensed matter

Features of the Faraday and Kerr magneto-optical effects in nanoscale Y$_3$Fe$_5$O$_{12}$ films and Gd$_3$Ga$_5$O$_{12}$, Nd$_3$Ga$_5$O$_{12}$ substrates

Yu. P. Sukhorukova, A. V. Telegina, I. D. Lobova, A. M. Korovinb

a Institute of Metal Physics, Ural Branch of the Russian Academy of Sciences, Yekaterinburg, Russia
b Ioffe Institute, St. Petersburg, Russia

Abstract: The Faraday and Kerr magneto-optical effects for ultra-thin films of yttrium iron garnet Y$_3$Fe$_5$O$_{12}$ and monocrystalline substrates Gd$_3$Ga$_5$O$_{12}$ and Nd$_3$Ga$_5$O$_{12}$ were studied in the visible spectrum range 1.3 eV $< E <$ 4.5 eV in fields up to 1 T. Verdet constants for the substrates Gd$_3$Ga$_5$O$_{12}$ (V $\approx$ +1048 min/(T $\cdot$ cm)) and Nd$_3$Ga$_5$O$_{12}$ ($\approx$ 4000 min/(T $\cdot$ cm)) were determined, and features of the Faraday and Kerr effects spectra related to the magneto-optical properties of the substrates for Y$_3$Fe$_5$O$_{12}$/ Gd$_3$Ga$_5$O$_{12}$ and Y$_3$Fe$_5$O$_{12}$/Nd$_3$Ga$_5$O$_{12}$ structures were identified. It was shown that, by excluding the contribution from the substrates, the spectral and field dependencies of the magneto-optical effects in nanoscale films correspond to the data for bulk Y$_3$Fe$_5$O$_{12}$. An estimation of the relaxation layer was carried out, and it was shown that nanoscale films, being comparable in thickness to the critical layer, can possess a specific Faraday rotation (15–20 deg/$\mu$m) close to that of bulk materials, demonstrating the high quality of the obtained samples.

Keywords: Faraday effect, Kerr effect, magneto-optics, YIG (yttrium iron garnet), films, interface.

Received: 31.05.2024
Revised: 29.07.2024
Accepted: 29.07.2024

DOI: 10.61011/OS.2024.07.58897.6245-24



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© Steklov Math. Inst. of RAS, 2025