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Optics and Spectroscopy, 2022 Volume 130, Issue 10, Pages 1491–1498 (Mi os1846)

Spectroscopy of condensed matter

Dielectric measurements of nanocrystalline VO$_2$ : Fe films

A. V. Ilinskiya, R. A. Castrob, V. A. Klimova, A. A. Kononovb, E. B. Shadrina

a Ioffe Institute, 194021 St. Petersburg, Russia
b Herzen State Pedagogical University of Russia, 191186 St. Petersburg, Russia

Abstract: Dielectric spectroscopy methods revealed the existence of two types of relaxation processes in the semiconductor phase of VO$_2$ : Fe films. The characteristic relaxation times are denoted by $\tau_1$ and $\tau_2$. It is shown that the temperature dependences of $\tau_1$ and $\tau_2$ have hysteresis, the position of the loops of which coincides with the points of the semiconductor-metal phase transition. in VO$_2$ : Fe films. $\tau_1$ corresponds to undoped, and $\tau_2$ corresponds to Fe-doped nanocrystallites of the VO$_2$ film. It is shown that the physical mechanism of the relaxation process is due to the establishment of equilibrium after the action of an electric field on conduction electrons. The numerical values of the parameters of the distribution of relaxers over relaxation times are determined.

Keywords: dielectric measurements, correlation effects, vanadium dioxide, VO$_2$, insulator-metal phase transition.

Received: 06.07.2022
Revised: 20.07.2022
Accepted: 20.07.2022

DOI: 10.21883/OS.2022.10.53618.3902-22



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