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Pisma v Zhurnal Tekhnicheskoi Fiziki, 2023 Volume 49, Issue 24, Pages 31–34 (Mi pjtf7151)

International Conference PhysicA.SPb/2023

Suppression of reverse reactions during carbon dioxide decomposition in microwave discharge plasma

N. V. Chekmarev, D. A. Mansfeld, E. I. Preobrazhensky, S. V. Sintsov, M. A. Remez, A. V. Vodopyanov

Federal Research Center A.V. Gaponov-Grekhov Institute of Applied Physics of the Russian Academy of Sciences, Nizhny Novgorod, Russia

Abstract: The paper investigates the decomposition of carbon dioxide (CO$_2$) in a plasma maintained by microwave radiation from a gyrotron at a frequency of 24 GHz in a waveguide plasmatron in a flow of argon and CO$_2$. An increase in the degree of CO$_2$ conversion and energy efficiency up to 2.5 times was demonstrated due to cooling (quenching) of the post-discharge region by a counterflow gas. It is shown that the cooling efficiency depends on the density and heat capacity of the quenching gas, and the maximum degree of conversion is achieved when nitrogen and argon are used as quenching gases.

Keywords: CO$_2$ conversion, atmospheric pressure discharge, gyrotron, qenching.

Received: 12.05.2023
Revised: 19.07.2023
Accepted: 30.10.2023

DOI: 10.61011/PJTF.2023.24.56868.89A



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